2 definitions found From The Collaborative International Dictionary of English v.0.48 [gcide]: Unshackle \Un*shac"kle\, v. t. [1st pref. un- + shackle.] To loose from shackles or bonds; to set free from restraint; to unfetter. --Addison. [1913 Webster] From Moby Thesaurus II by Grady Ward, 1.0 [moby-thes]: 33 Moby Thesaurus words for "unshackle": discharge, emancipate, liberate, loose, loosen, manumit, release, unbar, unbind, unbolt, unbridle, unbuckle, uncage, unchain, unfetter, ungag, unhandcuff, unhobble, unlash, unlatch, unleash, unlock, unloose, unloosen, unmanacle, unmuzzle, unpen, unpinion, unstrap, untether, untie, untruss, unyoke
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